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Nonlinear phase-field model for electrode-electrolyte interface evolution
L. Liang, Y. Qi, F. Xue, , S.J. Harris, L.-Q. Chen
Published in
2012
Volume: 86
   
Issue: 5
Abstract
A nonlinear phase-field model is proposed for modeling microstructure evolution during highly nonequilibrium processes. We consider electrochemical reactions at electrode-electrolyte interfaces leading to electroplating and electrode-electrolyte interface evolution. In contrast to all existing phase-field models, the rate of temporal phase-field evolution and thus the interface motion in the current model is considered nonlinear with respect to the thermodynamic driving force. It produces Butler-Volmer-type electrochemical kinetics for the dependence of interfacial velocity on the overpotential at the sharp-interface limit. At the low overpotential it recovers the conventional Allen-Cahn phase-field equation. This model is generally applicable to many other highly nonequilibrium processes where linear kinetics breaks down. © 2012 American Physical Society.
About the journal
JournalPhysical Review E - Statistical, Nonlinear, and Soft Matter Physics
ISSN15393755